alright, Dolphin - N64 is running a N64 game on the Virtual Console from Dolphin. You are correct that Dolphin is a GameCube emulator, but it is also able to emulate the Wii (you may be able to run Wii games on your computer, but I think the cpu may hold you back on a lot of games). As far as I know, you cannot add any quality enhancements this way, except for increasing resolution and AA/AF from Dolphin, and by running an emulator inside an emulator, it may have a performance cost.
As for the texture packs, there are not a huge assortment of them. The most common ones will be for the Zelda games, and depending on the pack, you will need to use a specific graphics plugin. Most require Rice's while others require Jabo's.
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http://textures.emulation64.com/index.php?id=downloads
This has a good assortment of packs, others can be found all over the internet. They do require some changes in the plugin settings to load the textures instead of the defaults, but they are pretty simple to find.
Disc-based systems can run the games from a few different sources. Almost all games can be run from a disc image, but can be burned to disc if you so choose. A few of the less-used formats may have to be either converted to a more common format, or can be mounted to a virtual drive the emulator can run it from.
My recommendations: GameCube/Wii-Dolphin, PSX-ePSXe, PS2-PCSX2. You can take a look here
viewtopic.php?f=10&t=4001 for some of the other PlayStation (PSX) emulators. As for a Saturn emulator, I am not familiar with these, so I cannot recommend one to you. You can also try some DreamCast games if you want to try them out, I hear Chankast and NullDC are pretty good. These all should be available on this site's emulator section.